AbstractWe have developed a new class of lanthanide nano clusters that self assemble using flexible Schiff base ligands. Cd Ln and Ni Ln clusters, [Ln8Cd24(L1)12(OAc)39Cl7(OH)2] (Ln = Nd, Eu), [Eu8Cd24(L1)12(OAc)44], [Ln8Cd24(L2)12(OAc)44] (Ln = Nd, Yb, Sm) and [Nd2Ni4(L3)2(acac)6(NO3)2(OH)2], were constructed using different types of flexible Schiff base ligands. These molecular nano clusters exhibit anisotropic architectures that differ considerably depending upon the presence of Cd (nano drum) or Ni (square like nano cluster).
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